Right now debating getting rid of a really nice highly modded STTNG and going all Stern. In a similar boat since I will have POTC and LOTR (picking it up in a week).
SM seems high right now. People are asking 5k for originals. Kinda hard to justify a game paying 5k for an 8 year old game when the new should hit for 6500 or less. Also expect price to drop as the remakes filter in. Some people will want the new, some people will want the old. Many won't care and go off condition/price. It is going to increase the suppy of SM so expect the value to drop a bit.
Seen some HUO TSPP's at 4500. Seems like a good deal relative to what LOTR goes for now. Has plenty of depth and a unique layout.
X-Men, just can't get past Wolverine. Seriously who thought making him that huge was a good idea? Yeah, you can go with the aftermarket captive ball, but dunno.
I would hold off on RBION. It is a great game, but in a small collection it has typical lawlor moves that won't set it apart from TZ. Others might chime in with TF or Avatar, but cannot get past the theme on either of them. In a big collection sure, but if you are going to stay small get what you want for play and theme.