Gert Frobe as Auric Goldfinger pasted_image (resized).png

As far as comedy villans:
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Brother Cavil from Battlestar Galactica: pasted_image (resized).png

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I'm the Juggernaut bitch!.gif

David Warner: The only TRON cast member that played three parts (Dillinger, SARK and The Master Control Program)
Villian trifecta!

Robin Williams as Walter Finch in the American remake of Insomnia:
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Another T.V. villian. Lord Commander from Final Space (Voiced by David Tennant).

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"... Draw ..."Man in Black.gif

The Chamberlain:
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"You don't Believe Me? You Will Doctor Jones. You will become a true believer!"

Mombi:

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Not that I cared for the movie that much, the cast was great in The Dark Tower.

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Matthew McConaughey as Walter